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Emerging S-Scheme Photocatalyst
Zhang, Liuyang; Zhang, Jianjun; Yu, Huogen; Yu, Jiaguo
2022-01
发表期刊ADVANCED MATERIALS
卷号34期号:11
原始文献类型Review ; Early Access
摘要Photocatalysis is a green technology to use ubiquitous and intermittent sunlight. The emerging S-scheme heterojunction has demonstrated its superiority in photocatalysis. This article covers the state-of-the-art progress and provides new insights into its general designing criteria. It starts with the challenges confronted by single photocatalyst from the perspective of energy dissipation by borrowing the common behaviors in the dye molecule. Subsequently, other problems faced by single photocatalyst are summarized. Then a viable solution for these problems is the construction of heterojunctions. To overcome the problems and mistakes of type-II and Z-scheme heterojunctions, S-scheme heterojunction is proposed and the underlying reaction mechanism is summarized. Afterward, the design principles for S-scheme heterojunction are proposed and four types of S-scheme heterojunctions are suggested. Following this, direct characterization techniques for testifying the charge transfer in S-scheme heterojunction are presented. Finally, different photocatalytic applications of S-scheme heterojunctions are summarized. Specifically, this work endeavors to clarify the critical understanding on curved Fermi level in S-scheme heterojunction interface, which can help strengthen and advance the fundamental theories of photocatalysis. Moreover, the current challenges and prospects of the S-scheme heterojunction photocatalyst are critically discussed.
关键词curved Fermi level design principle electron transfer photocatalytic fundamental S-scheme heterojunction
DOI10.1002/adma.202107668
语种英语
ISSN0935-9648
收录类别SCIE ; EI
EI入藏号20221111802847
WOS记录号WOS:000748794300001
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
出版者WEINHEIM
出版地WILEY-V C H VERLAG GMBH
EISSN1521-4095
引用统计
被引频次:981[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.cug.edu.cn/handle/2XU834YA/333310
专题中国地质大学(武汉)
作者单位China Univ Geosci, Lab Solar Fuel, Fac Mat Sci & Chem, 388 Lumo Rd, Wuhan 430074, Peoples R China
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GB/T 7714
Zhang, Liuyang,Zhang, Jianjun,Yu, Huogen,et al. Emerging S-Scheme Photocatalyst[J]. ADVANCED MATERIALS,2022,34(11).
APA Zhang, Liuyang,Zhang, Jianjun,Yu, Huogen,&Yu, Jiaguo.(2022).Emerging S-Scheme Photocatalyst.ADVANCED MATERIALS,34(11).
MLA Zhang, Liuyang,et al."Emerging S-Scheme Photocatalyst".ADVANCED MATERIALS 34.11(2022).
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